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Multi-wavelength Laser Absorption Spectroscopy for High-temperature Reaction Kinetics.

紀錄類型:	書目-電子資源 : Monograph/item
正題名/作者:	Multi-wavelength Laser Absorption Spectroscopy for High-temperature Reaction Kinetics./
作者:	Pinkowski, Nicolas H. .
出版者:	Ann Arbor : ProQuest Dissertations & Theses, : 2021,
面頁冊數:	161 p.
附註:	Source: Dissertations Abstracts International, Volume: 83-05, Section: B.
Contained By:	Dissertations Abstracts International83-05B.
標題:	Hydrocarbons. -
電子資源:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=28827994
ISBN:	9798494462480

Multi-wavelength Laser Absorption Spectroscopy for High-temperature Reaction Kinetics.
Pinkowski, Nicolas H. .

Multi-wavelength Laser Absorption Spectroscopy for High-temperature Reaction Kinetics. - Ann Arbor : ProQuest Dissertations & Theses, 2021 - 161 p.

Source: Dissertations Abstracts International, Volume: 83-05, Section: B.

Thesis (Ph.D.)--Stanford University, 2021.

This item must not be sold to any third party vendors.

This dissertation presents advanced measurement science that ultimately supports the design, development, and characterization of next-generation energy systems. Part I presents a mathematical framework and approach for measuring the composition of complex, reacting gaseous mixtures with multi-wavelength laser-absorption spectroscopy. Suites of laser systems were interfaced with shock tubes to measure the composition of mixtures during the pyrolysis of a single-component fuel (1-butene), alternative (carbon-neutral) jet fuel mixtures, and traditional jet fuels. These methods were established to help determine the time-dependent composition of complex high-temperature chemistry. With the framework of Part I in place, Part II presents work that increases the number of laser wavelengths used by a factor of 10, while reducing the hardware needed to acquire this extra information. The second part of this thesis adopts an emerging technology, known as dual-comb spectroscopy, for use in high-temperature reaction kinetic studies. This approach provides ultra-fast broadband absorption data used in a variety of conditions in the different chapters of Part II. Taken together, the two parts of this thesis provide a framework for characterizing complex and reacting high-temperature gas mixtures and introduce advanced tools that push the boundary of measurement capability.

ISBN: 9798494462480Subjects--Topical Terms:

697428
Hydrocarbons.

Multi-wavelength Laser Absorption Spectroscopy for High-temperature Reaction Kinetics.
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520 $a This dissertation presents advanced measurement science that ultimately supports the design, development, and characterization of next-generation energy systems. Part I presents a mathematical framework and approach for measuring the composition of complex, reacting gaseous mixtures with multi-wavelength laser-absorption spectroscopy. Suites of laser systems were interfaced with shock tubes to measure the composition of mixtures during the pyrolysis of a single-component fuel (1-butene), alternative (carbon-neutral) jet fuel mixtures, and traditional jet fuels. These methods were established to help determine the time-dependent composition of complex high-temperature chemistry. With the framework of Part I in place, Part II presents work that increases the number of laser wavelengths used by a factor of 10, while reducing the hardware needed to acquire this extra information. The second part of this thesis adopts an emerging technology, known as dual-comb spectroscopy, for use in high-temperature reaction kinetic studies. This approach provides ultra-fast broadband absorption data used in a variety of conditions in the different chapters of Part II. Taken together, the two parts of this thesis provide a framework for characterizing complex and reacting high-temperature gas mixtures and introduce advanced tools that push the boundary of measurement capability.
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