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Investigation of Carbonaceous Aeroso...

Olson, Michael R.

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Investigation of Carbonaceous Aerosol Optical Properties to Understand Impacts on Air Quality and Composition.

紀錄類型:	書目-電子資源 : Monograph/item
正題名/作者:	Investigation of Carbonaceous Aerosol Optical Properties to Understand Impacts on Air Quality and Composition./
作者:	Olson, Michael R.
出版者:	Ann Arbor : ProQuest Dissertations & Theses, : 2016,
面頁冊數:	218 p.
附註:	Source: Dissertation Abstracts International, Volume: 78-09(E), Section: B.
Contained By:	Dissertation Abstracts International78-09B(E).
標題:	Atmospheric sciences. -
電子資源:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10188285
ISBN:	9781369704730

Investigation of Carbonaceous Aerosol Optical Properties to Understand Impacts on Air Quality and Composition.
Olson, Michael R.

Investigation of Carbonaceous Aerosol Optical Properties to Understand Impacts on Air Quality and Composition. - Ann Arbor : ProQuest Dissertations & Theses, 2016 - 218 p.

Source: Dissertation Abstracts International, Volume: 78-09(E), Section: B.

Thesis (Ph.D.)--The University of Wisconsin - Madison, 2016.

The optical properties of carbonaceous aerosols were investigated to understand the impact source emissions and ambient particulate matter (PM) have on atmospheric radiative forcing. Black carbon (BC) is a strong absorber of visible light and contributes highly to atmospheric radiative forcing, therefore it is important to link BC properties to combustion emission sources. Brown carbon (BrC) is poorly understood and may be an important contributor to both positive and negative radiative forcing. The research investigates these primary knowledge gaps. The optical properties of carbonaceous aerosols were investigated to understand the impact source emissions and ambient particulate matter (PM) have on atmospheric radiative forcing. Black carbon (BC) is a strong absorber of visible light and contributes highly to atmospheric radiative forcing, therefore it is important to link BC properties to combustion emission sources. Brown carbon (BrC) is poorly understood and may be an important contributor to both positive and negative radiative forcing. The research investigates these primary knowledge gaps. Multiple methods were developed and applied to quantify the mass absorption cross-section (MAC) at multiple wavelengths of source and ambient samples. The MAC of BC was determined to be approximately 7.5 m2g-1 at 520nm. However, the MAC was highly variable with OC fraction and wavelength. The BrC MAC was similar for all sources, with the highest absorption in the UV at 370nm; the MAC quickly decreases at larger wavelengths. In the UV, the light absorption by BrC could exceed BC contribution by over 100 times, but only when the OC fraction is large (>90%) as compared to the total carbon. BrC was investigated by measuring the light absorption of solvent extracted fractions in water, dichloromethane, and methanol. Source emissions exhibited greater light absorption in methanol extractions as compared to water and DCM extracts. The BrC MAC was 2.4 to 3.7 m2g-1 at 370nm in methanol. Ambient samples showed similar MACs for the water and methanol extracts. Dichloromethane extracts did not have a significant light absorption characteristics for ambient samples. BrC and BC were measured in Beijing, China. Both were reduced significantly when restrictive air pollution controls were put in place. The industrial regions south and east of Beijing were the highest contributors to ambient BrC and BC. The controls reduced BrC more than BC as compared to observations during the regions heating period. Using the color characteristics of ambient PM, a model was developed to estimate elemental and organic carbon (EC/OC). The method will allow fast and cost effective quantification of PM composition in combination with large climate and health studies, especially in the developing world.

ISBN: 9781369704730Subjects--Topical Terms:

3168354
Atmospheric sciences.

Investigation of Carbonaceous Aerosol Optical Properties to Understand Impacts on Air Quality and Composition.
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