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Gas-Phase Ion Chemistry: Kinetics an...

Nichols, Charles M.

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Gas-Phase Ion Chemistry: Kinetics and Thermodynamics.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Gas-Phase Ion Chemistry: Kinetics and Thermodynamics./
Author:	Nichols, Charles M.
Published:	Ann Arbor : ProQuest Dissertations & Theses, : 2016,
Description:	162 p.
Notes:	Source: Dissertation Abstracts International, Volume: 77-10(E), Section: B.
Contained By:	Dissertation Abstracts International77-10B(E).
Subject:	Physical chemistry. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10108688
ISBN:	9781339720241

Gas-Phase Ion Chemistry: Kinetics and Thermodynamics.
Nichols, Charles M.

Gas-Phase Ion Chemistry: Kinetics and Thermodynamics. - Ann Arbor : ProQuest Dissertations & Theses, 2016 - 162 p.

Source: Dissertation Abstracts International, Volume: 77-10(E), Section: B.

Thesis (Ph.D.)--University of Colorado at Boulder, 2016.

This thesis employs gas-phase ion chemistry to study the kinetics and thermodynamics of chemical reactions and molecular properties. Gas-phase ion chemistry is important in diverse regions of the universe. It is directly relevant to the chemistry occurring in the atmospheres of planets and moons as well as the molecular clouds of the interstellar medium. Gas-phase ion chemistry is also employed to determine fundamental properties, such as the proton and electron affinities of molecules. Furthermore, gas-phase ion chemistry can be used to study chemical events that typically occur in the condensed-phase, such as prototypical organic reactions, in an effort to reveal the intrinsic properties and mechanisms of chemical reactions.

ISBN: 9781339720241Subjects--Topical Terms:

1981412
Physical chemistry.

Gas-Phase Ion Chemistry: Kinetics and Thermodynamics.
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020 $a 9781339720241
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035 $a AAI10108688
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100 1 $a Nichols, Charles M. $3 3281792
245 1 0 $a Gas-Phase Ion Chemistry: Kinetics and Thermodynamics.
260 1 $a Ann Arbor : $b ProQuest Dissertations & Theses, $c 2016
300 $a 162 p.
500 $a Source: Dissertation Abstracts International, Volume: 77-10(E), Section: B.
500 $a Advisers: Veronica M. Bierbaum; William C. Lineberger.
502 $a Thesis (Ph.D.)--University of Colorado at Boulder, 2016.
520 $a This thesis employs gas-phase ion chemistry to study the kinetics and thermodynamics of chemical reactions and molecular properties. Gas-phase ion chemistry is important in diverse regions of the universe. It is directly relevant to the chemistry occurring in the atmospheres of planets and moons as well as the molecular clouds of the interstellar medium. Gas-phase ion chemistry is also employed to determine fundamental properties, such as the proton and electron affinities of molecules. Furthermore, gas-phase ion chemistry can be used to study chemical events that typically occur in the condensed-phase, such as prototypical organic reactions, in an effort to reveal the intrinsic properties and mechanisms of chemical reactions.
520 $a Mass spectrometry is used to investigate the reactivity and fundamental properties of ions. Kinetic data for reactions between cations or anions with neutral atoms or molecules is acquired using the selected ion flow tube (SIFT). These data are interpreted mechanistically and thermodynamically using literature data and theoretical computations. Additionally, the proton affinities of a series of anions are determined using a triple quadrupole mass spectrometer by investigating the collision induced dissociation of proton-bound, anionic heterodimers.
520 $a The SIFT is coupled with a variety of ion-generation techniques. This thesis reports the design and operation of a new electrospray ion source for the SIFT in detail. The electrospray ionization technique allows ions that are pre-formed in the condensed-phase to be transmitted into the gas-phase for studies of their reactivity.
590 $a School code: 0051.
650 4 $a Physical chemistry. $3 1981412
650 4 $a Analytical chemistry. $3 3168300
690 $a 0494
690 $a 0486
710 2 $a University of Colorado at Boulder. $b Chemistry. $3 1019559
773 0 $t Dissertation Abstracts International $g 77-10B(E).
790 $a 0051
791 $a Ph.D.
792 $a 2016
793 $a English
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10108688