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Photocathode tunability: The photoem...

Velazquez, Daniel Gomez.

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Photocathode tunability: The photoemissive properties of ultra-thin multilayered MgO/Ag/MgO films synthesized by pulsed laser deposition.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Photocathode tunability: The photoemissive properties of ultra-thin multilayered MgO/Ag/MgO films synthesized by pulsed laser deposition./
Author:	Velazquez, Daniel Gomez.
Description:	183 p.
Notes:	Source: Dissertation Abstracts International, Volume: 76-12(E), Section: B.
Contained By:	Dissertation Abstracts International76-12B(E).
Subject:	Condensed matter physics. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3715703
ISBN:	9781321939859

Photocathode tunability: The photoemissive properties of ultra-thin multilayered MgO/Ag/MgO films synthesized by pulsed laser deposition.
Velazquez, Daniel Gomez.

Photocathode tunability: The photoemissive properties of ultra-thin multilayered MgO/Ag/MgO films synthesized by pulsed laser deposition. - 183 p.

Source: Dissertation Abstracts International, Volume: 76-12(E), Section: B.

Thesis (Ph.D.)--Illinois Institute of Technology, 2015.

Much of the early development of photocathode materials was aimed at the growth of photoemissive thin films with low work function, and high quantum efficiency (QE). It has been shown, both theoretically and experimentally, that metal-insulator junctions can lead to the modification of the work function and QE for coverages of a few monolayers of metal oxides on metallic substrates. However, the production of electron beams suitable for new photoinjector technologies often requires low emittance beams from the cathode itself.

ISBN: 9781321939859Subjects--Topical Terms:

3173567
Condensed matter physics.

Photocathode tunability: The photoemissive properties of ultra-thin multilayered MgO/Ag/MgO films synthesized by pulsed laser deposition.
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020 $a 9781321939859
035 $a (MiAaPQ)AAI3715703
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100 1 $a Velazquez, Daniel Gomez. $3 3193354
245 1 0 $a Photocathode tunability: The photoemissive properties of ultra-thin multilayered MgO/Ag/MgO films synthesized by pulsed laser deposition.
300 $a 183 p.
500 $a Source: Dissertation Abstracts International, Volume: 76-12(E), Section: B.
500 $a Adviser: Linda Spentzouris.
502 $a Thesis (Ph.D.)--Illinois Institute of Technology, 2015.
520 $a Much of the early development of photocathode materials was aimed at the growth of photoemissive thin films with low work function, and high quantum efficiency (QE). It has been shown, both theoretically and experimentally, that metal-insulator junctions can lead to the modification of the work function and QE for coverages of a few monolayers of metal oxides on metallic substrates. However, the production of electron beams suitable for new photoinjector technologies often requires low emittance beams from the cathode itself.
520 $a A theoretical model [Phys. Rev. Lett. 104, 046801 (2010)] based on a multilayered structure of MgO/Ag(001)/MgO with 4 monolayers of Ag(001) flanked by n monolayers (ML) of MgO indicates the possibility to reduce the surface work function and photoelectron beam emittance when the thickness n of the MgO layers is 2 or 3 monolayers. These predictions were tested experimentally. Synthesis of multilayered MgO/Ag/MgO films was performed using a custom-built pulsed laser deposition (PLD) system. In-situ growth monitoring was carried out by Reflection High-Energy Electron Diffraction (RHEED). Ex-situ techniques such as Scanning Tunneling Microscopy (STM), Scanning Electron Microscopy/Energy Dispersive Spectroscopy (EDS) and Photoelectron Spectroscopy (PES) were used to show the formation of the crystalline and chemical structure. A custom-built Kelvin Probe/photocurrent-detector system was used to measure the work function and QE of the samples. Angle Resolved Photoelectron Spectroscopy was used to measure the angular photoelectron yield. Simultaneous reduction of work function and increase of QE was observed for (001) oriented multilayers of various thicknesses with respect to that of a bare Ag/MgO(001) surface. Work function measurements of multilayers of various thicknesses in the (111) orientation also showed a monotonic reduction with respect to that of a bare Ag/Si(111) surface. Angular emission was compared for a MgO/Ag/MgO multilayer (thicknesses of 3 ML/4 ML/3 ML) sample and Ag/MgO(001). Emission analysis of the angle-resolved photoelectron spectra shows a net change in the angular emission with high kinetic energy electron density shifted toward surface-normal emission.
520 $a Experimental results were consistent with theoretical predictions, which open the promising possibility of customizing emission properties by direct manipulation of the surface band structure of the emitter.
590 $a School code: 0091.
650 4 $a Condensed matter physics. $3 3173567
650 4 $a Materials science. $3 543314
650 4 $a Nanoscience. $3 587832
690 $a 0611
690 $a 0794
690 $a 0565
710 2 $a Illinois Institute of Technology. $b Physics. $3 3193355
773 0 $t Dissertation Abstracts International $g 76-12B(E).
790 $a 0091
791 $a Ph.D.
792 $a 2015
793 $a English
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3715703