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Functional 2D nanoparticle/polymer a...

Xiong, Shisheng.

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Functional 2D nanoparticle/polymer array: Interfacial assembly, transfer, characterization, and coupling to photonic crystal cavities.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Functional 2D nanoparticle/polymer array: Interfacial assembly, transfer, characterization, and coupling to photonic crystal cavities./
Author:	Xiong, Shisheng.
Description:	149 p.
Notes:	Source: Dissertation Abstracts International, Volume: 72-12, Section: B, page: 7628.
Contained By:	Dissertation Abstracts International72-12B.
Subject:	Materials science. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3473654
ISBN:	9781124882307

Functional 2D nanoparticle/polymer array: Interfacial assembly, transfer, characterization, and coupling to photonic crystal cavities.
Xiong, Shisheng.

Functional 2D nanoparticle/polymer array: Interfacial assembly, transfer, characterization, and coupling to photonic crystal cavities. - 149 p.

Source: Dissertation Abstracts International, Volume: 72-12, Section: B, page: 7628.

Thesis (Ph.D.)--The University of New Mexico, 2011.

This item must not be sold to any third party vendors.

We developed a universal, facile and robust method to prepare free-standing, ordered and patternable nanoparticle/polymer monolayer arrays by evaporation-induced self-assembly at a fluid interface. The ultra-thin monolayer nanoparticle/polymer arrays are sufficiently robust that they can be transferred to arbitrary substrates, even with complex topographies. More importantly, the Poly (methyl methacrylate) (PMMA) in the system serves as a photoresist enabling two modes of electron beam (e-beam) nanoparticle patterning. These ultra-thin films of monolayer nanoparticle arrays are of fundamental interest as 2D artificial solids for electronic, magnetic and optical properties and are also of technological interest for a diverse range of applications in micro- and macro-scale devices including photovoltaics, sensors, catalysis, and magnetic storage. By co-assembly with block co-polymers, the nanoparticles were selectively positioned in one specific phase, representing a high throughput route for creating nanoparticle patterns. The self-assembly process was investigated by combined in-situ grazing incidence small angle x-ray scattering (GISAXS) and numerical simulation. By e-beam irradiation of free-standing 2D NP/polymer arrays, anisotropic nanowire arrays have been fabricated. Additionally, preliminary investigation on assembly of binary nanoparticle arrays has also been introduced, serving as promising future directions of interfacial assembly.

ISBN: 9781124882307Subjects--Topical Terms:

543314
Materials science.

Functional 2D nanoparticle/polymer array: Interfacial assembly, transfer, characterization, and coupling to photonic crystal cavities.
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020 $a 9781124882307
035 $a (MiAaPQ)AAI3473654
035 $a AAI3473654
040 $a MiAaPQ $c MiAaPQ
100 1 $a Xiong, Shisheng. $3 3175369
245 1 0 $a Functional 2D nanoparticle/polymer array: Interfacial assembly, transfer, characterization, and coupling to photonic crystal cavities.
300 $a 149 p.
500 $a Source: Dissertation Abstracts International, Volume: 72-12, Section: B, page: 7628.
500 $a Adviser: C. Jeffrey Brinker.
502 $a Thesis (Ph.D.)--The University of New Mexico, 2011.
506 $a This item must not be sold to any third party vendors.
506 $a This item must not be added to any third party search indexes.
520 $a We developed a universal, facile and robust method to prepare free-standing, ordered and patternable nanoparticle/polymer monolayer arrays by evaporation-induced self-assembly at a fluid interface. The ultra-thin monolayer nanoparticle/polymer arrays are sufficiently robust that they can be transferred to arbitrary substrates, even with complex topographies. More importantly, the Poly (methyl methacrylate) (PMMA) in the system serves as a photoresist enabling two modes of electron beam (e-beam) nanoparticle patterning. These ultra-thin films of monolayer nanoparticle arrays are of fundamental interest as 2D artificial solids for electronic, magnetic and optical properties and are also of technological interest for a diverse range of applications in micro- and macro-scale devices including photovoltaics, sensors, catalysis, and magnetic storage. By co-assembly with block co-polymers, the nanoparticles were selectively positioned in one specific phase, representing a high throughput route for creating nanoparticle patterns. The self-assembly process was investigated by combined in-situ grazing incidence small angle x-ray scattering (GISAXS) and numerical simulation. By e-beam irradiation of free-standing 2D NP/polymer arrays, anisotropic nanowire arrays have been fabricated. Additionally, preliminary investigation on assembly of binary nanoparticle arrays has also been introduced, serving as promising future directions of interfacial assembly.
520 $a Controlling the rate of spontaneous emission and thus promoting the photon generation efficiency is a key step toward fabrication of Quantum dot based single-photon sources, and harnessing of light energy from emitters with a broad emitting spectrum. Coupling of photo emitters to photonic cavities without perturbing the optical performance of cavities remains as a challenge in study of Purcell effect based on quantum electrodynamics. Taking advantage of interfacial assembly and transfer, we have achieved controlled deposition of quantum dots into high Q photonic microcavities and studied the modification of their optical properties. Anomalous enhanced spontaneous emission and Fabry-Perot resonance have been observed.
590 $a School code: 0142.
650 4 $a Materials science. $3 543314
650 4 $a Nanoscience. $3 587832
690 $a 0794
690 $a 0565
710 2 $a The University of New Mexico. $b Chemical Engineering. $3 2094212
773 0 $t Dissertation Abstracts International $g 72-12B.
790 $a 0142
791 $a Ph.D.
792 $a 2011
793 $a English
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3473654