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Framework materials for solar energy...

Wang, Cheng.

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Framework materials for solar energy utilization.

紀錄類型:	書目-語言資料,印刷品 : Monograph/item
正題名/作者:	Framework materials for solar energy utilization./
作者:	Wang, Cheng.
面頁冊數:	208 p.
附註:	Source: Dissertation Abstracts International, Volume: 74-12(E), Section: B.
Contained By:	Dissertation Abstracts International74-12B(E).
標題:	Chemistry, General. -
電子資源:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3593287
ISBN:	9781303358036

Framework materials for solar energy utilization.
Wang, Cheng.

Framework materials for solar energy utilization. - 208 p.

Source: Dissertation Abstracts International, Volume: 74-12(E), Section: B.

Thesis (Ph.D.)--The University of North Carolina at Chapel Hill, 2013.

The ever-increasing global demand for energy has stimulated a new wave of research activities on generating clean and renewable energy using sunlight. Following the molecular approach adopted by green plants, scientists have developed various molecular systems that are capable of converting photons to high energy redox equivalents, as well as molecular catalysts for both water oxidation and proton/CO2 reduction. There are however not efficient ways of assembling these functional molecular components into hierarchical organizations to convert sunlight energy into chemical energy.

ISBN: 9781303358036Subjects--Topical Terms:

1021807
Chemistry, General.

Framework materials for solar energy utilization.
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502 $a Thesis (Ph.D.)--The University of North Carolina at Chapel Hill, 2013.
520 $a The ever-increasing global demand for energy has stimulated a new wave of research activities on generating clean and renewable energy using sunlight. Following the molecular approach adopted by green plants, scientists have developed various molecular systems that are capable of converting photons to high energy redox equivalents, as well as molecular catalysts for both water oxidation and proton/CO2 reduction. There are however not efficient ways of assembling these functional molecular components into hierarchical organizations to convert sunlight energy into chemical energy.
520 $a Metal-organic frameworks (MOFs) are a class of crystalline materials that are constructed from well-defined molecular building blocks and metal-cluster connecting nodes. Similarly, crosslinked polymers (CPs) are built from well-designed organic precursors and represent a new class of robust materials. These framework materials provide a potential platform to organize different molecular components to achieve artificial photosynthesis. In this thesis, I will report our efforts on assembling MOFs and CPs for light harvesting, water oxidation, and photocatalytic proton and CO2 reduction. These materials not only provide a unique opportunity to integrate different functional molecular components hierarchically for energy conversion or organic transformation, but also allow the elucidation of molecular mechanisms for related reactions.
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