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Modeling of a hydrogenated vacuum ga...
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Govindhakannan, Jagannathan.
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Modeling of a hydrogenated vacuum gas oil hydrocracker.
紀錄類型:
書目-電子資源 : Monograph/item
正題名/作者:
Modeling of a hydrogenated vacuum gas oil hydrocracker./
作者:
Govindhakannan, Jagannathan.
面頁冊數:
115 p.
附註:
Source: Dissertation Abstracts International, Volume: 64-03, Section: B, page: 1368.
Contained By:
Dissertation Abstracts International64-03B.
標題:
Engineering, Chemical. -
電子資源:
http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3083379
ISBN:
0496311883
Modeling of a hydrogenated vacuum gas oil hydrocracker.
Govindhakannan, Jagannathan.
Modeling of a hydrogenated vacuum gas oil hydrocracker.
- 115 p.
Source: Dissertation Abstracts International, Volume: 64-03, Section: B, page: 1368.
Thesis (Ph.D.)--Texas Tech University, 2003.
Hydrocracking is used in the petroleum industry to convert low-quality feedstocks into highly-valued transportation fuels such as gasoline, diesel, and jet fuel. Hydrocracking is usually carried out in two stages. The first stage decomposes sulfur and nitrogen-containing compounds and hydrogenates the aromatics. The liquid fraction from the first stage is hydroisomerized and hydrocracked in the second stage. The primary objective of the present research is to develop a very detailed, fundamental, and molecular-level model for the second stage hydrocracking process.
ISBN: 0496311883Subjects--Topical Terms:
1018531
Engineering, Chemical.
Modeling of a hydrogenated vacuum gas oil hydrocracker.
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Thesis (Ph.D.)--Texas Tech University, 2003.
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Hydrocracking is used in the petroleum industry to convert low-quality feedstocks into highly-valued transportation fuels such as gasoline, diesel, and jet fuel. Hydrocracking is usually carried out in two stages. The first stage decomposes sulfur and nitrogen-containing compounds and hydrogenates the aromatics. The liquid fraction from the first stage is hydroisomerized and hydrocracked in the second stage. The primary objective of the present research is to develop a very detailed, fundamental, and molecular-level model for the second stage hydrocracking process.
520
$a
The modeling methodologies reported in the literature for the hydrocracking process thus far, describe the feed and product compositions based on the boiling range and the actual reaction network is reduced to a smaller number of reactions between the lumped species. The present approach applies the concept of single event kinetics to the hydrocracking process. In this approach, the various reactions involved in hydrocracking are considered in terms of fundamental elementary steps involving carbocations.
520
$a
A computer algorithm, in which feed and product molecules, carbocations, and olefinic intermediates are represented by means of Boolean relation matrices and characterization vectors has been developed to generate the elementary reaction networks for paraffinic, naphthenic, and aromatic feed components. The standardized labeling algorithms for acyclic and cyclic hydrocarbon structures are developed. The network generation leads to a very large network of elementary reactions (>106). However, due to the molecular nature of the approach, the number of rate parameters is kept within the tractable limits (<30) and the rate parameters are independent of the feedstock composition.
520
$a
Since the number of chemical species generated in the reaction network is very large, a certain degree of lumping is required to reduce the number of continuity equations for the components to be integrated along the reactor. The lumps should be chosen in terms of the present day analytical capabilities. The single event kinetic model, in the present work, considers the pure components and lumps according to the carbon number. Each lump is defined by its carbon number and the type of chemical structure that represents that lump. The type of chemical structures considered here are n-paraffins, iso-paraffins, mono-, di-, tri-, and tetra-naphthenes, mono-, di-, tri-, and tetra-aromatics, and naphtheno-mono-, naphtheno-di-, and naphtheno-tri-aromatics. Some lumps are individual molecules while most are collection of molecules. For the lump involving a collection of molecules, the properties of the lump are determined by averaging of the properties of each individual molecule comprising the lump.
520
$a
The model parameters are estimated from the synthetic product distribution data obtained from an industrial organization. A partially hydrogenated vacuum gas oil (VGO) is considered as the feedstock. The single event kinetic model is inserted into a homogeneous reactor model and the resulting continuity equations are integrated numerically along the length of the catalyst bed. The reactor simulation results are the temperature profile, composition profiles, and hydrogen consumption profile through the catalyst bed. The hydrogen consumption is calculated in a very rigorous way in the single event model, which is not possible with the lumped models. The reactor simulation results are consistent with industrial practice and published information.
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http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3083379
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