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Cold Thallium Fluoride Beam : = Buffer Gas Cooling, Beam Production, and B Triplet Pi Excited State Hyperfine Spectra.
紀錄類型:
書目-電子資源 : Monograph/item
正題名/作者:
Cold Thallium Fluoride Beam :/
其他題名:
Buffer Gas Cooling, Beam Production, and B Triplet Pi Excited State Hyperfine Spectra.
作者:
Edwards, Eustace R.
面頁冊數:
1 online resource (310 pages)
附註:
Source: Dissertations Abstracts International, Volume: 85-01, Section: B.
Contained By:
Dissertations Abstracts International85-01B.
標題:
Molecular physics. -
電子資源:
http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=30310365click for full text (PQDT)
ISBN:
9798379762186
Cold Thallium Fluoride Beam : = Buffer Gas Cooling, Beam Production, and B Triplet Pi Excited State Hyperfine Spectra.
Edwards, Eustace R.
Cold Thallium Fluoride Beam :
Buffer Gas Cooling, Beam Production, and B Triplet Pi Excited State Hyperfine Spectra. - 1 online resource (310 pages)
Source: Dissertations Abstracts International, Volume: 85-01, Section: B.
Thesis (Ph.D.)--Yale University, 2023.
Includes bibliographical references
The possibility of laser cooling on thallium fluoride's (TlF) |X1Σ> → |B3Π> optical transition has generated renewed interest in the use of TlF in fundamental physical measurements. In particular, researchers were interested in the hyperfine structure in the lowest rotational energy levels of the B state, and the laser cooling potential of lowest Q-branch transition. In this work, we constructed and characterized a cryogenic buffer gas beam source (CBGBS) to produce a rotationally cold TlF beam (3.6K). Using the cold beam, we recorded low temperature hyperfine spectra, and discovered the B state possesses hyperfine interaction (roughly 4 times the size of the rotational constant), which leads to rotational state mixing, and spoiling of the initially proposed laser cooling transition. Since the cold beam provided unambiguous identification of TlF's Q branch transitions, we were able to perform preliminary transverse laser cooling on the proposed laser cooling transitions.
Electronic reproduction.
Ann Arbor, Mich. :
ProQuest,
2023
Mode of access: World Wide Web
ISBN: 9798379762186Subjects--Topical Terms:
3174737
Molecular physics.
Subjects--Index Terms:
Buffer gasIndex Terms--Genre/Form:
542853
Electronic books.
Cold Thallium Fluoride Beam : = Buffer Gas Cooling, Beam Production, and B Triplet Pi Excited State Hyperfine Spectra.
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Source: Dissertations Abstracts International, Volume: 85-01, Section: B.
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Advisor: DeMille, David;Lamoreaux, Steve.
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Thesis (Ph.D.)--Yale University, 2023.
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The possibility of laser cooling on thallium fluoride's (TlF) |X1Σ> → |B3Π> optical transition has generated renewed interest in the use of TlF in fundamental physical measurements. In particular, researchers were interested in the hyperfine structure in the lowest rotational energy levels of the B state, and the laser cooling potential of lowest Q-branch transition. In this work, we constructed and characterized a cryogenic buffer gas beam source (CBGBS) to produce a rotationally cold TlF beam (3.6K). Using the cold beam, we recorded low temperature hyperfine spectra, and discovered the B state possesses hyperfine interaction (roughly 4 times the size of the rotational constant), which leads to rotational state mixing, and spoiling of the initially proposed laser cooling transition. Since the cold beam provided unambiguous identification of TlF's Q branch transitions, we were able to perform preliminary transverse laser cooling on the proposed laser cooling transitions.
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