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Synthetic Studies toward Ent-Kaurene...

Billett, Brent Allen.

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Synthetic Studies toward Ent-Kaurene Natural Products: An Application of Carbon-Carbon Bond Activation in Synthesis.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Synthetic Studies toward Ent-Kaurene Natural Products: An Application of Carbon-Carbon Bond Activation in Synthesis./
Author:	Billett, Brent Allen.
Published:	Ann Arbor : ProQuest Dissertations & Theses, : 2020,
Description:	235 p.
Notes:	Source: Dissertations Abstracts International, Volume: 82-01, Section: B.
Contained By:	Dissertations Abstracts International82-01B.
Subject:	Organic chemistry. -
Online resource:	https://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=27955571
ISBN:	9798662397149

Synthetic Studies toward Ent-Kaurene Natural Products: An Application of Carbon-Carbon Bond Activation in Synthesis.
Billett, Brent Allen.

Synthetic Studies toward Ent-Kaurene Natural Products: An Application of Carbon-Carbon Bond Activation in Synthesis. - Ann Arbor : ProQuest Dissertations & Theses, 2020 - 235 p.

Source: Dissertations Abstracts International, Volume: 82-01, Section: B.

Thesis (Ph.D.)--The University of Chicago, 2020.

This item is not available from ProQuest Dissertations & Theses.

Recent work in the area of transition metal catalyzed carbon-carbon (C-C) σ-bond activation has allowed for new strategic bond disconnection. Toward this end, the Dong lab has developed a Rh(I)-catalyzed C-C bond activation/olefin insertion strategy to access highly polycyclic scaffolds found in natural products. Of specific interest are the ent-kaurenes eriocalyxin B and isodonal. Herein, we disclose our synthetic efforts toward the family through a C-C activation method. Other key steps in the synthesis include a tandem Birch reduction propargylation reaction as well as a carbon-oxygen bond cleavage/lactonization sequence.

ISBN: 9798662397149Subjects--Topical Terms:

523952
Organic chemistry.
Subjects--Index Terms:

Carbon-carbon activation

Synthetic Studies toward Ent-Kaurene Natural Products: An Application of Carbon-Carbon Bond Activation in Synthesis.
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100 1 $a Billett, Brent Allen. $3 3564235
245 1 0 $a Synthetic Studies toward Ent-Kaurene Natural Products: An Application of Carbon-Carbon Bond Activation in Synthesis.
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300 $a 235 p.
500 $a Source: Dissertations Abstracts International, Volume: 82-01, Section: B.
500 $a Advisor: Dong, Guangbin.
502 $a Thesis (Ph.D.)--The University of Chicago, 2020.
506 $a This item is not available from ProQuest Dissertations & Theses.
506 $a This item must not be sold to any third party vendors.
520 $a Recent work in the area of transition metal catalyzed carbon-carbon (C-C) σ-bond activation has allowed for new strategic bond disconnection. Toward this end, the Dong lab has developed a Rh(I)-catalyzed C-C bond activation/olefin insertion strategy to access highly polycyclic scaffolds found in natural products. Of specific interest are the ent-kaurenes eriocalyxin B and isodonal. Herein, we disclose our synthetic efforts toward the family through a C-C activation method. Other key steps in the synthesis include a tandem Birch reduction propargylation reaction as well as a carbon-oxygen bond cleavage/lactonization sequence.
590 $a School code: 0330.
650 4 $a Organic chemistry. $3 523952
653 $a Carbon-carbon activation
653 $a Ent-kaurene
653 $a Natural product
653 $a Synthesis
690 $a 0490
710 2 $a The University of Chicago. $b Chemistry. $3 1675066
773 0 $t Dissertations Abstracts International $g 82-01B.
790 $a 0330
791 $a Ph.D.
792 $a 2020
793 $a English
856 4 0 $u https://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=27955571