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Optical Activity Anisotropy in Solids.

Martin, Alexander T.

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Optical Activity Anisotropy in Solids.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Optical Activity Anisotropy in Solids./
Author:	Martin, Alexander T.
Published:	Ann Arbor : ProQuest Dissertations & Theses, : 2018,
Description:	267 p.
Notes:	Source: Dissertation Abstracts International, Volume: 80-03(E), Section: B.
Contained By:	Dissertation Abstracts International80-03B(E).
Subject:	Physical chemistry. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10845247
ISBN:	9780438634824

Optical Activity Anisotropy in Solids.
Martin, Alexander T.

Optical Activity Anisotropy in Solids. - Ann Arbor : ProQuest Dissertations & Theses, 2018 - 267 p.

Source: Dissertation Abstracts International, Volume: 80-03(E), Section: B.

Thesis (Ph.D.)--New York University, 2018.

Francois Arago first observed chromatic phenomena associated with optical rotatory dispersion of light along the high symmetry, optic axis of crystalline quartz in 1811. In the following two centuries, comparable measurements along low symmetry directions in solid materials have challenged Science. Though our understanding of the underlying physical principles that govern light polarization transformation has improved, the practical difficulties involved in solid state measurements have led to significant error and misunderstanding in the literature. This thesis serves as an update on the progress in the field of crystal optics, corrects some common misconceptions in the literature, and develops emerging techniques for measuring chiroptical properties in crystals and fabricated materials. Modern polarimeters employed in this work use complex polarization modulation schemes to recover the full normalized Mueller matrix, the transformation matrix which encodes all information related to linear optical phenomenon. A comprehensive methodology for the accurate measurement of optical tensors in crystalline media is developed here, incorporating recent technological advances in instrumentation sensitivity, methods for enhancement of the gyrotropic effect, variable coherence optical models, and the development of machine learning algorithms for smart starting guesses of optical parameters. Developing a robust and varied catalogue of optical tensors in anisotropic crystals will expand the range of materials used in optical device fabrication and characterization and help theoreticians bridge the elusive gap of structure-property relations. Here, we present measurements of optical activity anisotropy in crystals, fabricated metamaterials, and multilayer samples, and correlate these measurements to microscopic and macroscopic structure.

ISBN: 9780438634824Subjects--Topical Terms:

1981412
Physical chemistry.

Optical Activity Anisotropy in Solids.
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245 1 0 $a Optical Activity Anisotropy in Solids.
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300 $a 267 p.
500 $a Source: Dissertation Abstracts International, Volume: 80-03(E), Section: B.
500 $a Adviser: Bart Kahr.
502 $a Thesis (Ph.D.)--New York University, 2018.
520 $a Francois Arago first observed chromatic phenomena associated with optical rotatory dispersion of light along the high symmetry, optic axis of crystalline quartz in 1811. In the following two centuries, comparable measurements along low symmetry directions in solid materials have challenged Science. Though our understanding of the underlying physical principles that govern light polarization transformation has improved, the practical difficulties involved in solid state measurements have led to significant error and misunderstanding in the literature. This thesis serves as an update on the progress in the field of crystal optics, corrects some common misconceptions in the literature, and develops emerging techniques for measuring chiroptical properties in crystals and fabricated materials. Modern polarimeters employed in this work use complex polarization modulation schemes to recover the full normalized Mueller matrix, the transformation matrix which encodes all information related to linear optical phenomenon. A comprehensive methodology for the accurate measurement of optical tensors in crystalline media is developed here, incorporating recent technological advances in instrumentation sensitivity, methods for enhancement of the gyrotropic effect, variable coherence optical models, and the development of machine learning algorithms for smart starting guesses of optical parameters. Developing a robust and varied catalogue of optical tensors in anisotropic crystals will expand the range of materials used in optical device fabrication and characterization and help theoreticians bridge the elusive gap of structure-property relations. Here, we present measurements of optical activity anisotropy in crystals, fabricated metamaterials, and multilayer samples, and correlate these measurements to microscopic and macroscopic structure.
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