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Selective and Catalytic Hydrodeoxyge...

Klein, Ian Michael.

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Selective and Catalytic Hydrodeoxygenation of Lignin in Model Compounds and Intact Biomass.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Selective and Catalytic Hydrodeoxygenation of Lignin in Model Compounds and Intact Biomass./
Author:	Klein, Ian Michael.
Published:	Ann Arbor : ProQuest Dissertations & Theses, : 2015,
Description:	131 p.
Notes:	Source: Dissertation Abstracts International, Volume: 77-04(E), Section: B.
Contained By:	Dissertation Abstracts International77-04B(E).
Subject:	Chemistry. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3736248
ISBN:	9781339251295

Selective and Catalytic Hydrodeoxygenation of Lignin in Model Compounds and Intact Biomass.
Klein, Ian Michael.

Selective and Catalytic Hydrodeoxygenation of Lignin in Model Compounds and Intact Biomass. - Ann Arbor : ProQuest Dissertations & Theses, 2015 - 131 p.

Source: Dissertation Abstracts International, Volume: 77-04(E), Section: B.

Thesis (Ph.D.)--Purdue University, 2015.

With persistent volatility in crude oil prices and an increased awareness of global climate change, the case for use of bio-renewable resources in production of liquid fuels and chemicals is compelling. A major obstacle in the efficient conversion of biomass to useful chemicals and fuels lies in the recalcitrant nature of lignocellulosic biomass and the lack of a selective process for the conversion of lignin to a useful product stream. We have studied a Pd/C and ZnII system for the catalytic depolymerization of a wide variety of wood lignin, in yields up to 54%, and selectively upgraded the resulting monolignols into 4-propylguaiacol and 4-propylsyringol. Herein we present a detailed study of the hydrodeoxygenation of lignin, including a mechanistic investigation into the synergistic Pd/C and ZnII system through use of both model lignin compounds and lignocellulosic biomass.

ISBN: 9781339251295Subjects--Topical Terms:

516420
Chemistry.

Selective and Catalytic Hydrodeoxygenation of Lignin in Model Compounds and Intact Biomass.
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245 1 0 $a Selective and Catalytic Hydrodeoxygenation of Lignin in Model Compounds and Intact Biomass.
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300 $a 131 p.
500 $a Source: Dissertation Abstracts International, Volume: 77-04(E), Section: B.
500 $a Adviser: Mahdi M. Abu-Omar.
502 $a Thesis (Ph.D.)--Purdue University, 2015.
520 $a With persistent volatility in crude oil prices and an increased awareness of global climate change, the case for use of bio-renewable resources in production of liquid fuels and chemicals is compelling. A major obstacle in the efficient conversion of biomass to useful chemicals and fuels lies in the recalcitrant nature of lignocellulosic biomass and the lack of a selective process for the conversion of lignin to a useful product stream. We have studied a Pd/C and ZnII system for the catalytic depolymerization of a wide variety of wood lignin, in yields up to 54%, and selectively upgraded the resulting monolignols into 4-propylguaiacol and 4-propylsyringol. Herein we present a detailed study of the hydrodeoxygenation of lignin, including a mechanistic investigation into the synergistic Pd/C and ZnII system through use of both model lignin compounds and lignocellulosic biomass.
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