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The Discovery, Development, and Mech...

Dang, Hester.

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The Discovery, Development, and Mechanistic Investigations of Transition Metal-Catalyzed Organic Reactions.

Record Type:	Electronic resources : Monograph/item
Title/Author:	The Discovery, Development, and Mechanistic Investigations of Transition Metal-Catalyzed Organic Reactions./
Author:	Dang, Hester.
Published:	Ann Arbor : ProQuest Dissertations & Theses, : 2016,
Description:	193 p.
Notes:	Source: Dissertation Abstracts International, Volume: 78-01(E), Section: B.
Contained By:	Dissertation Abstracts International78-01B(E).
Subject:	Organic chemistry. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10138638
ISBN:	9781339941950

The Discovery, Development, and Mechanistic Investigations of Transition Metal-Catalyzed Organic Reactions.
Dang, Hester.

The Discovery, Development, and Mechanistic Investigations of Transition Metal-Catalyzed Organic Reactions. - Ann Arbor : ProQuest Dissertations & Theses, 2016 - 193 p.

Source: Dissertation Abstracts International, Volume: 78-01(E), Section: B.

Thesis (Ph.D.)--University of Washington, 2016.

Organic reactions have wide spread applications in drug development, chemical biology, and materials science. However, traditional chemical techniques can be inefficient i.e., low yields and/or poor selectivity, for constructing structurally complex motifs and for selectively activating strong bonds. To address these problems, there has been an increasing focus on developing new organic reactions catalyzed by transition metals.

ISBN: 9781339941950Subjects--Topical Terms:

523952
Organic chemistry.

The Discovery, Development, and Mechanistic Investigations of Transition Metal-Catalyzed Organic Reactions.
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100 1 $a Dang, Hester. $3 3281067
245 1 4 $a The Discovery, Development, and Mechanistic Investigations of Transition Metal-Catalyzed Organic Reactions.
260 1 $a Ann Arbor : $b ProQuest Dissertations & Theses, $c 2016
300 $a 193 p.
500 $a Source: Dissertation Abstracts International, Volume: 78-01(E), Section: B.
500 $a Adviser: Gojko Lalic.
502 $a Thesis (Ph.D.)--University of Washington, 2016.
520 $a Organic reactions have wide spread applications in drug development, chemical biology, and materials science. However, traditional chemical techniques can be inefficient i.e., low yields and/or poor selectivity, for constructing structurally complex motifs and for selectively activating strong bonds. To address these problems, there has been an increasing focus on developing new organic reactions catalyzed by transition metals.
520 $a This document describes my contributions to transition metal catalysis and includes the following works: 1) Catalytic activation of a single C-F bond in trifluoromethyl arenes for the synthesis of difluoromethyl arenes, 2) Mild copper-catalyzed fluorination of alkyl triflates using potassium fluoride, 3) Copper-catalyzed reduction of alkyl triflates and iodides: an efficient method for the deoxygenation of primary and secondary alcohols, 4) Synthesis of hindered anilines, and 5) Synthesis of tertiary alkyl amines from terminal alkenes: copper-catalyzed amination of alkyl boranes. For each work, I will describe its significance to organic synthesis, its discovery and development, and the investigation of its mechanism.
590 $a School code: 0250.
650 4 $a Organic chemistry. $3 523952
690 $a 0490
710 2 $a University of Washington. $b Chemistry. $3 2093573
773 0 $t Dissertation Abstracts International $g 78-01B(E).
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856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10138638