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Operando research in heterogeneous c...

Frenken, Joost.

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Operando research in heterogeneous catalysis

紀錄類型:	書目-電子資源 : Monograph/item
正題名/作者:	Operando research in heterogeneous catalysis/ edited by Joost Frenken, Irene Groot.
其他作者:	Frenken, Joost.
出版者:	Cham :Springer International Publishing : : 2017.,
面頁冊數:	xiv, 222 p. :ill., digital ;24 cm.
內容註:	From the Contents: Scanning probe microscopy under high-pressure conditions -- Surface X-ray diffraction under high-pressure conditions -- Ambient pressure X-ray photoelectron spectroscopy -- Planar laser-induced fluorescence.
Contained By:	Springer eBooks
標題:	Heterogeneous catalysis. -
電子資源:	http://dx.doi.org/10.1007/978-3-319-44439-0
ISBN:	9783319444390

Operando research in heterogeneous catalysis
Operando research in heterogeneous catalysis[electronic resource] /edited by Joost Frenken, Irene Groot. - Cham :Springer International Publishing :2017. - xiv, 222 p. :ill., digital ;24 cm. - Springer series in chemical physics,v.1140172-6218 ;. - Springer series in chemical physics ;v.114..

From the Contents: Scanning probe microscopy under high-pressure conditions -- Surface X-ray diffraction under high-pressure conditions -- Ambient pressure X-ray photoelectron spectroscopy -- Planar laser-induced fluorescence.

This book is devoted to the emerging field of techniques for visualizing atomic-scale properties of active catalysts under actual working conditions, i.e. high gas pressures and high temperatures. It explains how to understand these observations in terms of the surface structures and dynamics and their detailed interplay with the gas phase. This provides an important new link between fundamental surface physics and chemistry, and applied catalysis. The book explains the motivation and the necessity of operando studies, and positions these with respect to the more traditional low-pressure investigations on the one hand and the reality of industrial catalysis on the other. The last decade has witnessed a rapid development of new experimental and theoretical tools for operando studies of heterogeneous catalysis. The book has a strong emphasis on the new techniques and illustrates how the challenges introduced by the harsh, operando conditions are faced for each of these new tools. Therefore, one can also read this book as a collection of recipes for the development of operando instruments. At present, the number of scientific results obtained under operando conditions is still limited and mostly focused on a simple test reaction, the catalytic oxidation of CO. This reaction thus forms a natural binding element between the chapters, linking the demonstrations of new techniques, and also connecting the theoretical and experimental studies. Some first results on other reactions are also presented. If there is one thing that can be concluded already in this early stage, it is that the catalytic conditions themselves can have dramatic effects on the structure and composition of the surfaces of catalysts, which, in turn can greatly affect the mechanisms, the activity, and the selectivity of the chemical reactions that they catalyze.

ISBN: 9783319444390

Standard No.: 10.1007/978-3-319-44439-0doiSubjects--Topical Terms:

726833
Heterogeneous catalysis.

LC Class. No.: QD505

Dewey Class. No.: 541.395

Operando research in heterogeneous catalysis
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520 $a This book is devoted to the emerging field of techniques for visualizing atomic-scale properties of active catalysts under actual working conditions, i.e. high gas pressures and high temperatures. It explains how to understand these observations in terms of the surface structures and dynamics and their detailed interplay with the gas phase. This provides an important new link between fundamental surface physics and chemistry, and applied catalysis. The book explains the motivation and the necessity of operando studies, and positions these with respect to the more traditional low-pressure investigations on the one hand and the reality of industrial catalysis on the other. The last decade has witnessed a rapid development of new experimental and theoretical tools for operando studies of heterogeneous catalysis. The book has a strong emphasis on the new techniques and illustrates how the challenges introduced by the harsh, operando conditions are faced for each of these new tools. Therefore, one can also read this book as a collection of recipes for the development of operando instruments. At present, the number of scientific results obtained under operando conditions is still limited and mostly focused on a simple test reaction, the catalytic oxidation of CO. This reaction thus forms a natural binding element between the chapters, linking the demonstrations of new techniques, and also connecting the theoretical and experimental studies. Some first results on other reactions are also presented. If there is one thing that can be concluded already in this early stage, it is that the catalytic conditions themselves can have dramatic effects on the structure and composition of the surfaces of catalysts, which, in turn can greatly affect the mechanisms, the activity, and the selectivity of the chemical reactions that they catalyze.
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